There have been a few threads of late discussing Titans, so I thought it was probably about time we attempted to gather what information we could on the Loyalist and Traitor Legions that were around during the Heresy and beforehand. I did some research a while back as I was thinking about what Legion and colour scheme to use when I got round to adding Titans in support of my Epic Thousand Sons, so here is what I managed to find - almost all of it is shamelessly cribbed from Lexicanum at this stage. Any further information people have will be welcomed - bear in mind, of course, that much of this information is very old background indeed, so is not hugely reliable, but still is probably useful...
Known LegionsDeath StalkersAlignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: Battle for Mars
Colour Scheme: ?
Famous Titans: ?
Source: WD 110, Codex:Eye of Terror,
MechanicumLegio Magna (Flaming Skulls)Alignment during the Heresy: Traitor - Khorne
Homeworld: ?
Notable Actions: Attack on the Imperial Palace
Colour Scheme: Red/orange/yellow/black

Famous Titans: ?
Source: Adeptus Titanicus, Collected Visions, Imperial Armour 1,
MechanicumLegio Astorum (Warp Runners)Alignment during the Heresy: Imperial
Homeworld: Lucius
Notable Actions: Fought the Legio Mortis on Tallarn
Colour Scheme: blue, flame decoration

Famous Titans: Fortuna Imperiatrix, fought on Tallarn
Source: Adeptus Titanicus, Imperial Armour 1
Legio Ignatium (Fire Wasps)Alignment during the Heresy: Imperial
Homeworld: Mars
Notable Actions: Battle for Mars, Defence of the Imperial Palace, Sarosh
Colour Scheme: Black & red, decoration in yellow

Famous Titans: Imperious Prima, a Warmonger Titan involved in the defence of the palace and dating from before the foundation of the Imperium.
Source: Adeptus Titanicus, Collected Visions, The Descent of Angels,
MechanicumLegio Gryphonicus (War Gryphons)Alignment during the Heresy: Imperial
Homeworld: Gryphonne IV
Notable Actions: Yarrant III
Colour Scheme: yellow & grey

Famous Titans: ?
Source: Adeptus Titanicus, Imperial Armour 1
Legio Metallica (Iron Skulls)Alignment during the Heresy: Imperial
Homeworld: Metallica
Notable Actions: Centuries of combat against the ork empires surrounding Metallica before it was brought into the Imperium
Colour Scheme: Red, chevrons in white/black/yellow

Famous Titans: ?
Sources: Adeptus Titanicus, Imperial Armour 1
Legio Mortis (Deaths Heads)Alignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: Battle for Mars, Siege of the Imperial Palace, Tallarn, Istvaan III, Davin's Moon, Ullanor, Murder.
Colour Scheme: Black, red, silver, gold

Famous Titans: Dies Irae, an Imperator titan involved on Istvaan III. Vulkus Tor, destroyed by Orks on Ullanor. Deaths Head and Xestor's Sword, Warlord titans involved on Davin's Moon. Venator, a Warhound titan. Deaths Head Scouts, a Warhound titan formation that fought during the Heresy. Aquila Ignis, Imperator Titan destroyed on Mars in the battle for Magma City.
Source: Adeptus Titanicus, False Gods, Galaxy in Flames, Flight of the Eisenstein,
MechanicumLegio Victorum (Foe Slayers)Alignment during the Heresy: Imperial
Homeworld: Mars (heresy period), later Triplex Phall
Notable Actions: First Titans of the Legion were still based on Mars awaiting transport to other warzones when the battle for Mars began. Fought on Mars until they could be withdrawn to Terra. Took part in the Siege of the Imperial Palace.
Colour Scheme: Blue w. gold/bronze/yellow details

Famous Titans: Primus Malachi, a Reaver Titan that was the first Titan of the Legion to be completed. Imperious Cathedra, an Imperator Titan completed just before the Legion evacuated Mars.
Source: Adeptus Titanicus, Imperial Armour 1
Legio Vulcanum (The Dark Fire)Alignment during the Heresy: Traitor
Homeworld: Stygies VIII
Notable Actions: Stygies VIII had two Legions formed there due to its proximity to the Eye of Terror, Legio Vulcanum I and Legio Vulcanum II. During the heresy these Legions defected to Horus and were involved in a longrunning battle with Loyalist elements on their homeworld. Eventually both Legions were defeated with the aid of Eldar from Saim Hann and fled to the Eye of Terror at the end of the Heresy.
Colour Scheme: Olive Green, details in Yellow/Black
Famous Titans:
Venataris Mori, operated with the Night Lords Legion during the infamous purging of the Shi'Hu'Gal Dominion during the Great Crusade
Personnel: ?
Source: Adeptus Titanicus, Imperial Armour 1 & 6
Legio VulturumAlignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: ?
Colour Scheme: Silver, white, black
Famous Titans: ?
Source: Adeptus Titanicus, Adeptus Titanicus II
Legio TempestusAlignment during the Heresy: Imperial
Homeworld: Mars
Notable Actions: Epsiloid Binary Cluster wars, Battle for Mars. The bulk of the Legio is with Guilliman's crusade fleets when the Heresy breaks out.
Colour Scheme: Cobalt Blue
Famous Titans: Deus Tempestus, Warlord and first Titan of the Legio. Victorix Magna and Tharsis Hastatis, Warlords. Arcadia Fortis, Metallus Cebrenia - Reavers. Vulpus Rex, Raptoria, Astrus Lux - Warhounds.
Source:
MechanicumLegio Tempestor (Storm Lords)Alignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: Involved in the Siege of the Imperial Palace
Colour Scheme: Blue/Grey/Black & white checks

Famous Titans: ?
Personnel: ?
Source: Adeptus Titanicus, Collected Visions
Tiger EyesAlignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: ?
Colour Scheme: Yellow/black

Famous Titans: ?
Source: Adeptus Titanicus
Legio Damnatus (Warped Dogs)Alignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: The Legion's landing craft was destroyed while attempting to land on Terra during Horus' primary assault and the Legion was wiped out.
Colour Scheme: ?
Famous Titans: ?
Source: Collected Visions
Legio Astramana (Morning Stars)Alignment during the Heresy: Imperial
Homeworld: Graia
Notable Actions: ?
Colour Scheme: Green & yellow, decoration in white & black

Famous Titans: ?
Source: Adeptus Titanicus, Imperial Armour 1
Legio XerxesAlignment during the Heresy: ?
Homeworld: Mars
Notable Actions: Nurth
Colour Scheme: ?
Famous Titans: ?
Source:
LegionLegio Honorum (Death Bolts)Alignment during the Heresy: Imperial
Homeworld: Estaban VII, later Stygies VIII
Notable Actions: ?
Colour Scheme: Red & Gold, decoration in blue & silver
Famous Titans: ?
Source: Adeptus Titanicus, Imperial Armour 1,
MechanicumLegio Destructor (Steel Beasts)Alignment during the Heresy: Imperial
Homeworld: Accatran
Notable Actions: ?
Colour Scheme: ?
Famous Titans: ?
Source: Adeptus Titanicus II, Imperial Armour 1,
MechanicumBurning StarsAlignment during the Heresy: Traitor
Homeworld: ?
Notable Actions: Fought the Legio Ignatium dcuring the battle for Mars.
Colour Scheme: ?
Famous Titans: ?
Source:
MechanicumSo, if anyone can find any further information on Pre-heresy/Heresy era Titan Legions, any further sources that support or contradict what we know already, or anything else that might be useful, fire away!